Lithium–sulfur batteries are a promising energy-storage technology due to their relatively low cost and high theoretical energy density. However, one of their major technical problems is the shuttling of soluble polysulfides between electrodes, resulting in rapid capacity fading. Here, we present a metal–organic framework (MOF)-based battery separator to mitigate the shuttling problem. We show that the MOF-based separator acts as an ionic sieve in lithium–sulfur batteries, which selectively sieves Li+ ions while e ciently suppressing undesired polysulfides migrating to the anode side. When a sulfur-containing mesoporous carbon material (approximately 70 wt% sulfur content) is used as a cathode composite without elaborate synthesis or surface modification, a lithium–sulfur battery with a MOF-based separator exhibits a low capacity decay rate (0.019% per cycle over 1,500 cycles). Moreover, there is almost no capacity fading after the initial 100 cycles. Our approach demonstrates the potential for MOF-based materials as separators for energy-storage applications.
上传时间: 2017-11-23
上传用户:653357637
PDF打印程序,安装和使用都非常方便,而且支持各种操作系统。我已在好几种系统中用过
标签: PDF打印
上传时间: 2019-01-11
上传用户:pau008
2018专升本操作系统综合实践题目参考
上传时间: 2019-06-17
上传用户:aaaaa123
Accurate pose estimation plays an important role in solution of simultaneous localization and mapping (SLAM) problem, required for many robotic applications. This paper presents a new approach called R-SLAM, primarily to overcome systematic and non-systematic odometry errors which are generally caused by uneven floors, unexpected objects on the floor or wheel-slippage due to skidding or fast turns.The hybrid approach presented here combines the strengths of feature based and grid based methods to produce globally consistent high resolution maps within various types of environments.
标签: localization environments challenging Resilient mapping R-SLAM and in
上传时间: 2019-09-15
上传用户:zhudx2007
The concept of “smart city” is often used implying that the reader has a clear and common notion of what it means. However, in the current literature it is very hard to find a precise definition. What is even more interesting, it is not so easy to find a precise definition of what a city is.
标签: Facilitating Developing Designing Cities Smart
上传时间: 2020-05-25
上传用户:shancjb
Without conceding a blemish in the first edition, I think I had best come clean and admit that I embarked on a second edition largely to adopt a more geometric approach to the detection of signals in white Gaussian noise. Equally rigorous, yet more intuitive, this approach is not only student-friendly, but also extends more easily to the detection problem with random parameters and to the radar problem
标签: Communication Foundation Digital in
上传时间: 2020-05-26
上传用户:shancjb
In this paper, we consider the channel estimation problem in Millimeter wave (mmWave) wireless systems with large antenna arrays. By exploiting the inherent sparse nature of the mmWave channel, we develop a novel rate-adaptive channel estimation (RACE) algorithm, which can adaptively adjust the number of required channel measurements based on an expected probability of estimation error (PEE).
标签: Estimation Millimeter Adaptive Approach Channel Systems Rate MIMO Wave for
上传时间: 2020-05-26
上传用户:shancjb
Evolutionary Computation (EC) deals with problem solving, optimization, and machine learning techniques inspired by principles of natural evolution and ge- netics. Just from this basic definition, it is clear that one of the main features of the research community involved in the study of its theory and in its applications is multidisciplinarity. For this reason, EC has been able to draw the attention of an ever-increasing number of researchers and practitioners in several fields.
标签: Applications Evolutionary Computing of
上传时间: 2020-05-26
上传用户:shancjb
The objective of this book is to allow the reader to predict the received signal power produced by a particular radio transmitter. The first two chapters examine propagation in free space for point-to-point and point-to-area transmission, respectively. This is combined with a dis- cussion regarding the characteristics of antennas for various purposes. In chapter 3, the effect of obstacles, whether buildings or mountains, is discussed and analytical methods, whereby the strength of a signal is the shadow of an obstacle can be predicted, are presented.
标签: Propagation Essentials Radio Wave of
上传时间: 2020-05-27
上传用户:shancjb
In cellular networks, it is estimated that 2 3 of calls and over 90% of data services occur indoors. However, some surveys show that many households and businesses experience a poor indoor coverage problem. It has been identified that poor coverage is the main reason for churn, which is very costly for operators in saturated markets. How to provide good indoor coverage cost effectively is thus a demanding challenge for operators.
标签: Technologies Femtocells Deployment and
上传时间: 2020-05-27
上传用户:shancjb